"You dare threaten me, Thor, with so puny a weap-" ~tasered~
Bonus points for the hilarious irony of the god of thunder being dropped by a taser.
Selvig and Jane's shock and Darcy's line afterwards put the cherry on top of it all. "What? He was freaking me out!"
"YOU ARE NO MATCH FOR THE MIGHTY-" ~injected~
In the butt. Nose smooshed against the glass, with "squeeeek" sound effect as his face slides down the window. And absolutely perfect expression on Hemsworth's face.
Jane running over Thor - twice. "I'm really sorry, I'm not doing this on purpose!"
The best part was while Jane was being worried about subduing Thor if they need to, Darcy is checking her taser.
Thor: This drink, I like it! ANOTHER!! *hurls mug to the floor*
God of Thunder walks into a pet store. God of Thunder demands a horse. Possibly the best moment in the entire movie.
Thor: I NEED A HORSE!
Pet Shop Owner: We don't have horses. Just dogs, cats and birds.
Thor: Then give me one of those large enough to ride.
The delivery makes it even funnier than it sounds. Just look at how earnest Hemsworth's face is when he says it.
Not to mention that that scene clearly contains 2011's best Puppy Reaction Shot. Yes, that's right--as Thor comes striding into the shop, a number of adorable puppies look over curiously and this troper laughs to the point of tears every time. The shop owner's expression of sheer, unadulterated "What the hell just happened?" is only the icing on the cake.
Darcy: Whoa! Does he need CPR? 'Cause I TOTALLY know CPR.
When Thor is freaking out:
Thor: Hammer?! Hammer?!
Darcy: Yes, we know you're hammered... kind of obvious.
When they're at the diner:
Darcy: How could you eat a whole box of pop tarts and still be this hungry?
And in that scene, she takes a photo of him and says "This is goin' on Facebook, smile!" And he does. Just totally goes with it and grins dorkily. It's awesome.
And of course:
Darcy: You know, for a crazy homeless person he's prettycut.
And when Jane explains to the hospital staff that Darcy was the one who tasered Thor. Darcy gives a matter-of-fact "Yes, I did!"
SHIELD agents seeing the Warrior's Three and Sif walking down the street:
Even better, they can't figure out how to describe Volstagg...
"FOUND YOOOOOOU~!"
And their big, dopey grins when they're tapping on the glass. It's just adorable.
Made even better by Jane, Darcy and Erik's reactions. Three dumbfounded stares and Erik and Darcy actually drop their coffee in shock. At the same time !
Hawkeye's few lines are CMOF.
Hawkeye: Want me to slow him down sir, or you sending in more guys for him to beat up?
Hawkeye: You better call it, Coulson, 'cause I'm startin' to root for this guy.
Erik's conversation with Coulson.
How did an MD tear through an entire camp of highly-trained SHIELD agents? "Steroids!"
When it seems like they are about to get away.
Coulson: ...and Mr. Selvig? Keep him away from the bars.
Erik: I will.
...
Thor: Where are we going?
Erik: To get a drink.
Immediately after that, Thor and Selvig drinking. There's a deleted scene on the DVD at the bar where Selvig imitates Thor by smashing his mug of beer and demanding "ANOTHER!" They both say it and then the bartender repeats it and gives them another mug. Seconds later, they're going back to Jane's trailer and singing a song.
This ends with Thor toting the unconscious Selvig back to Jane's. "We drank, we fought, he made his ancestors proud."
Even funnier, his character is credited as "Stan The Man".
Hell. The whole scene surrounding the hammer's crater was pure win: the locals set up a tailgating party while everyone tries to lift Mjölnir.
Guy holding a beer: My turn.
Thor's rousing speech when it comes to Sif.
Thor: And who proved that a maiden had a place in battle, above all objections?
Sif:I did.
Thor: ...well, yes. But I supported you!
Early on there is an extremely tense face off with Thor, Loki, Sif, and the Warriors Three deep in enemy territory, one poorly-chosen word away from getting killed and starting a war. Loki manages to convince Laufey to let them depart safely, then this happens:
Frost Giant Soldier: (to Thor) "Run home little Princess."
The SHIELD agents first spot the Destroyer, but mistake him for another Iron Man prototype. Easy assumption to make, the poor guys!
Agent: Is it one of Stark's?
Coulson: I don't know. The guy never tells me anything.
From the deleted scenes, Loki you-have-to-be-kidding face when discovers that his plans are out of control because Thor has signed him in for that little trip to Jotunheim.
Then there's Sif and the Warriors Three deciding to go against Loki and try to find Thor on Earth. They approach Heimdall, fully expecting to face one of the greatest of badasses. When they tell him their plan, he simply says "Good" and goes along with it.
Heimdall: I am bound by honor to our king! I cannot open the bridge to you!
Fandral: ... complicated fellow, isn't he?
A small moment when Loki negotiates with Laufey, as he offers to trade them back the Casket of Ancient Winters to return Jotunheim to its former... extended awkward pause... glory.
It's definitely not MEANT to be funny, and in fact is an excellent example of the phrase 'inarticulate rage': when Loki tries to intervene in Odin and Thor's post Jotunheim screaming match, Odin just ROARS at him and Loki immediately shuts up. It's pretty hilarious.
The best part is that that roar wasn't in the script.
When Thor sets Mjölnir on top of Loki, effectively pinning him down. The sheer genius of it is what made me lose it the first time.
Agent Coulson: It's not easy to do what you did. You made my men—some of the most highly trained professionals in the world—look like a bunch of minimum-wage mall cops. That's hurtful.